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Multifunctional materials are key in organic (opto)electronics.However,their practical use requires the optimization of the self-assembly of multimodular architectures at surfaces using non-conventional methods,their controlled manipulation and responsiveness to external stimuli,and the quantitative study of various physico-chemical properties at distinct length-and time-scales.My lecture will review recent results we obtained on:(i) Development of novel processing and post processing methods to produces highly ordered supramolecular electroactive architectures.[1]